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(Salen)Mn-catalyzed epoxidation of alkenes: A two-zone process with different spin-state channels as suggested by DFT study

  1. Author:
    Abashkin, Y. G.
    Burt, S. K.

  2. Author Address

    Abashkin YG NCI, SAIC Frederick Inc, Adv Biomed Comp Ctr, Frederick, MD 21702 USA NCI, SAIC Frederick Inc, Adv Biomed Comp Ctr, Frederick, MD 21702 USA NCI, SAIC Frederick Inc, Adv Biomed Comp Ctr, Frederick, MD 21702 USA
    1. Year: 2004
    2. Date: Jan
  2. Journal: Organic Letters
    1. 6
    2. 1
    3. Pages: 59-62
  4. Type of Article: Article
  1. Abstract:

    A novel (two-zone process with different spin-state channels) mechanistic picture for the Jacobsen-Katsuki reaction is presented that provides insight into the still elusive understanding of the epoxidation mechanism. For the first time, we show that the salen moiety of the catalyst can be explicitly involved in the epoxidation process

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External Sources

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  2. DOI: 10.1021/ol036051t
  3. PMID: 14703350

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